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Dual Rh(II)/Pd(0) Relay Catalysis for One-Pot Synthesis of α-Quaternary Allylated Indolin-2-ones and Benzofuran-2-ones
- Authors
- Lee, Yu Lim; Lee, Kyu Ree; Xuan, Zi; Lee, Sang-gi
- Issue Date
- Mar-2021
- Publisher
- WILEY-V C H VERLAG GMBH
- Keywords
- Dual catalysis; Rhodium catalyst; Palladium catalyst; Indolin‐ 2‐ ones; Benzofuran‐ 2‐ ones
- Citation
- BULLETIN OF THE KOREAN CHEMICAL SOCIETY, v.42, no.3, pp 537 - 541
- Pages
- 5
- Indexed
- SCIE
SCOPUS
KCI
- Journal Title
- BULLETIN OF THE KOREAN CHEMICAL SOCIETY
- Volume
- 42
- Number
- 3
- Start Page
- 537
- End Page
- 541
- ISSN
- 0253-2964
1229-5949
- Abstract
- Cooperative Rh(II) and Pd(0) dual relay catalysis has been developed, which allowed one-pot synthesis of alpha-quaternary allylated indolin-2-ones and benzofuran-2-ones. The catalytic reaction proceeded through the sequential Rh(II)-catalyzed intramolecular aromatic C(sp(2))-H bond functionalization of alpha-diazo carbonyl compounds, followed by Pd(0)-catalyzed allylic alkylation with allylic carbonates to afford the products in high yields (up to 97%).
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