Two TPD-Based Conjugated Polymers: Synthesis and Photovoltaic Applications as Donor Materials
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초록

Two conjugated thienopyrrolodione-thiophene-vinyl-thiophene (TPDTVT)-based polymers, with one of them having an additional cyano (CN) group attached to the TVT building block, are synthesized and incorporated in photovoltaic device as electron-donating materials. Both TPD-TVT and TPD-TVTCN showed good thermal stability and appropriate solubility in chlorinated solvents, but they exhibited quite different optoelectrochemical and photovoltaic properties. The stronger intermolecular interactions of TPD-TVTCN, compared to TPD-TVT, lead to enhanced aggregation in blends with PC71BM. The domain sizes within 15-20 nm and improved molecular packing in TPD-TVTCN:PC71BM blend films result in better photovoltaic performance of TPD-TVTCN:PC71BM device compared to the device employing TPD-TVT.

키워드

bulk heterojunction solar cellspolymer solar cellspolymer donorsthienopyrrolodioneblend morphologyOPEN-CIRCUIT VOLTAGEORGANIC SOLAR-CELLSHIGH HOLE MOBILITYCOPOLYMERSEFFICIENCYACCEPTOR
제목
Two TPD-Based Conjugated Polymers: Synthesis and Photovoltaic Applications as Donor Materials
저자
Lee, Ji EunKim, Yu JinHong, JisuWu, XinweiHwang, Moon ChanKwon, Soon-KiAn, Tae KyuKim, Yun-Hi
DOI
10.1007/s13233-019-7015-8
발행일
2018-12
유형
Article
저널명
Macromolecular Research
26
13
페이지
1193 ~ 1199