A Thiacalix Basket and Its Anion-Dependent 2-D and 3-DSilver(I) Coordination Polymers via Exo-Coordination

A Thiacalix <i>Basket</i> and Its Anion-Dependent 2-D and 3-D Silver(I) Coordination Polymers via Exo-Coordination
  • Ju, Huiyeong
  • Park, In-Hyeok
  • Lee, Eunji
  • Kim, Chungsik
  • Kim, Seulgi
  • ... Lee, Shim Sung
  • 외 2명
Citations

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Citations

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7

초록

Thiacalix[4]arene-bis-1,2;3,4-crown-2 (basket or L) was isolated. Herein we report the first examples of the calix basket complexes. The combination of the basket and silver(I) salts afforded anion-dependent coordination polymers with different dimensionalities. The AgClO4 complex 1, {[Ag-2(L)(CH3OH)(ClO4)(2)]center dot 4CHCl(3)}(n) has a 2-D square-grid network, in which silver(I) atoms link the baskets to form a 1-D ribbon and these are crosslinked by perchlorate ions. While, the AgPF6 complex 2, {[Ag(L)(CH3OH)](PF6)}(n) exhibits a multichannel type 3-D framework with nbo-a topology. Since the basket acts as an ideal exo-coordinating S-4-platform, the topologies of both products are highly sensitive to the anion coordination.

키워드

CalixarenesMolecular basketsSilverCoordination polymersexo-CoordinationTOPOLOGICAL ANALYSISSTRUCTURAL-ANALYSISALKALI-METALNETWORKSMACROCYCLESCOMPLEXESDERIVATIVESDESIGN
제목
A Thiacalix Basket and Its Anion-Dependent 2-D and 3-DSilver(I) Coordination Polymers via Exo-Coordination
제목 (타언어)
A Thiacalix <i>Basket</i> and Its Anion-Dependent 2-D and 3-D Silver(I) Coordination Polymers via Exo-Coordination
저자
Ju, HuiyeongPark, In-HyeokLee, EunjiKim, ChungsikKim, SeulgiKuwahara, ShunsukeHabata, YoichiLee, Shim Sung
DOI
10.1002/ejic.201901216
발행일
2020-01
유형
Article
저널명
European Journal of Inorganic Chemistry
2020
4
페이지
356 ~ 360