Chemoselective synthesis of aryl(pyridinyl)methanol derivatives through Ni-NIXANTPHOS catalyzed alpha-arylation and tandem arylation/rearrangement of pyridylmethyl ethers

  • 김병선; 
  • Liu, ZF (Liu, Zhengfen); 
  • Li, MY (Li, Minyan); 
  • Wang, BJ (Wang, Bijun); 
  • Deng, GG (Deng, Guogang); 
  • 외 4명

초록

An efficient synthesis of aryl(pyridyl)-methanol derivatives using a nickel-NIXANTPHOS catalyst is described. Combinations of the Ni-NIXANTPHOS catalyst, solvent, and reaction temperature achieved chemoselective arylation and tandem arylation/rearrangement of pyridylmethyl ethers. A large variety of aryl halides were tolerated (55 examples, up to 96% yield). The scalability of the reaction is demonstrated. The order of the tandem arylation and [1,2]-Wittig rearrangement was probed by comparative studies.

제목
Chemoselective synthesis of aryl(pyridinyl)methanol derivatives through Ni-NIXANTPHOS catalyzed alpha-arylation and tandem arylation/rearrangement of pyridylmethyl ethers
저자
김병선; Liu, ZF (Liu, Zhengfen);  Li, MY (Li, Minyan);  Wang, BJ (Wang, Bijun);  Deng, GG (Deng, Guogang);  Chen, W (Chen, Wen);  Zhang, HB (Zhang, Hongbin);  Yang, XD (Yang, Xiaodong);  Walsh, PJ (Walsh, Patrick J.)
발행일
2018-06
저널명
Organic Chemistry Frontiers
권
5
호
12
페이지
1870 ~ 1876