Synthesis and Anion Recognition Features of a Molecular Cage Containing Both Hydrogen Bond Donors and Acceptors

  • Oh, Ju Hyun
  • Kim, Jeong Hyeon
  • Kim, Dong Sub
  • Han, Hye Jin
  • Lynch, Vincent M.
  • ... Kim, Sung Kuk
  • 외 1명
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초록

A molecular cage, macrobicycle 2, containing amide and pyrrole groups as hydrogen-bonding donors and imine groups as hydrogen-bonding acceptors has been synthesized. Compound 2 was found to recognize tetrahedral oxyanions with high affinities, such as H2PO4-, HSO4-, SO42-, and HP2O73-, as well as the spherical halide anions, in chloroform. A single-crystal X-ray diffraction analysis revealed that compound 2 formed a 1:1 complex with H2PO4- in the solid state.

키워드

RECEPTOR CHEMISTRY HIGHLIGHTSSELECTIVITYGUESTSOLD
제목
Synthesis and Anion Recognition Features of a Molecular Cage Containing Both Hydrogen Bond Donors and Acceptors
저자
Oh, Ju HyunKim, Jeong HyeonKim, Dong SubHan, Hye JinLynch, Vincent M.Sessler, Jonathan L.Kim, Sung Kuk
DOI
10.1021/acs.orglett.9b01515
발행일
2019-06-07
유형
Article
저널명
Organic Letters
21
11
페이지
4336 ~ 4339