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Rh(II)-Catalyzed C-N Bond Formation Using Enynones and N-H Imines: An Approach to Diarylmethylamines

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dc.contributor.authorCho, Ho-Jun-
dc.contributor.authorKim, Ye Lim-
dc.contributor.authorKim, Ju Hyun-
dc.date.accessioned2023-01-05T00:55:01Z-
dc.date.available2023-01-05T00:55:01Z-
dc.date.issued2022-12-
dc.identifier.issn0022-3263-
dc.identifier.issn1520-6904-
dc.identifier.urihttps://scholarworks.gnu.ac.kr/handle/sw.gnu/30010-
dc.description.abstractA Rh(II)-catalyzed furyl carbene N-H insertion reaction involving an N-sp2-hybridized imine is described, which represents an atom-economical route by which to access diarylmethylamine derivatives with high efficiency and broad substrate scope. An unusual reaction mechanism is proposed, in which the rhodium catalyst plays a dual role in facilitating enynone cyclization via activation and enhancement of the nucleophilicity of the NH imine.-
dc.format.extent12-
dc.language영어-
dc.language.isoENG-
dc.publisherAmerican Chemical Society-
dc.titleRh(II)-Catalyzed C-N Bond Formation Using Enynones and N-H Imines: An Approach to Diarylmethylamines-
dc.typeArticle-
dc.publisher.location미국-
dc.identifier.doi10.1021/acs.joc.2c02119-
dc.identifier.scopusid2-s2.0-85143528203-
dc.identifier.wosid000893109900001-
dc.identifier.bibliographicCitationThe Journal of Organic Chemistry, v.87, no.24, pp 16424 - 16435-
dc.citation.titleThe Journal of Organic Chemistry-
dc.citation.volume87-
dc.citation.number24-
dc.citation.startPage16424-
dc.citation.endPage16435-
dc.type.docTypeArticle-
dc.description.isOpenAccessN-
dc.description.journalRegisteredClassscie-
dc.description.journalRegisteredClassscopus-
dc.relation.journalResearchAreaChemistry-
dc.relation.journalWebOfScienceCategoryChemistry, Organic-
dc.subject.keywordPlusCATALYZED REGIOSELECTIVE ARYLATION-
dc.subject.keywordPlusINSERTION REACTIONS-
dc.subject.keywordPlusCOUPLING REACTIONS-
dc.subject.keywordPlusONE-POT-
dc.subject.keywordPlusALKYNES-
dc.subject.keywordPlusACTIVATION-
dc.subject.keywordPlusCARBENES-
dc.subject.keywordPlusACCESS-
dc.subject.keywordPlusFURANS-
dc.subject.keywordPlusOXIDATION-
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